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Low-temperature spectroscopy of the (C2H2)-C-12 (upsilon(1) + upsilon(3)) band in a helium buffer gas

  Articoli su Riviste JCR/ISI  (anno 2015)

Autori:  Santamaria L., Di Sarno V., Ricciardi I., De Rosa M., Mosca S., Santambrogio G., Maddaloni P., De Natale P

Affiliazione Autori:  CNR-INO, Istituto Nazionale di Ottica, Via Campi Flegrei 34, I-80078 Pozzuoli, Italy CNR-INO, Istituto Nazionale di Ottica, Via N. Carrara 1, I-50019 Sesto Fiorentino, Italy Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany INFN, Istituto Nazionale di Fisica Nucleare, Sez. di Firenze, Via G. Sansone 1, I-50019 Sesto Fiorentino, Italy CNR-INO, Istituto Nazionale di Ottica, Largo E. Fermi 6, I-50125 Firenze, Italy

Riassunto:  Buffer gas cooling with a He-4 gas is used to perform laser-absorption spectroscopy of the (C2H2)-C-12 (upsilon(1) + upsilon(3)) band at cryogenic temperatures. Doppler thermometry is first carried out to extract translational temperatures from the recorded spectra. Then, rotational temperatures down to 20 K are retrieved by fitting the Boltzmann distribution to the relative intensities of several ro-vibrational lines. The potential of our setup to tune the thermal equilibrium between translational and rotational degrees of freedom is also demonstrated. This can be used to reproduce in a controlled way the regime of non-local thermal equilibrium typically encountered in the interstellar medium. The underlying helium-acetylene collisional physics, relevant for modeling planetary atmospheres, is also addressed. In particular, the diffusion time of (C2H2)-C-12 in the buffer cell is measured against the He-4 flux at two separate translational temperatures; the observed behavior is then compared with that predicted by a Monte Carlo simulation, thus providing an estimate for the respective total elastic cross sections: sigma(el)(100 K) = (4 +/- 1) x 10(-20) m(2) and sigma(el)(25 K) = (7 +/- 2) x 10(-20) m(2).

Volume n.:  801 (1)      Pagine da: 50  a: 50
Ulteriori informazioni:  The authors acknowledge technical support by G. Notariale. This work was funded by MIUR-FIRB project RBFR1006TZ and by INFN project SUPREMO.
DOI: 10.1088/0004-637X/801/1/50

*Impact Factor della Rivista: (2015) 5.909   *Citazioni: 6
data tratti da "WEB OF SCIENCE" (marchio registrato di Thomson Reuters) ed aggiornati a:  26/05/2019

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