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Broadband Vibrational Cooling of Cold Cesium Molecules: Theory and Experiments

  Articoli su Riviste JCR/ISI  (anno 2009)

Autori:  Sofikitis D., Fioretti A., Weber S., Viteau M., Chotia A., Horchani R., Allegrini M., Chatel B., Comparat D., Pillet P

Affiliazione Autori:  Laboratoire Aime Cotton, CNRS, Universite Paris-Sud, Bat. 505, 91405 Orsay, France; Laboratoire Collisions, Agregats, Reactivite (UMR 5589, CNRS-Universite Paul Sabatier Toulouse 3), IRSAMC, Toulouse, France; CNISM, Dipartimento di Fisica, Universita di Pisa, Largo Pontecorvo, 356127 PISA, Italy

Riassunto:  The use of a broadband, frequency shaped femtosecond laser on translationally cold cesium molecules has recently demonstrated to be a very efficient method of cooling also the vibrational degree of freedom. A sample of cold molecules, initially distributed over several vibrational levels, has thus been transfered into a single selected vibrational level of the singlet. X(1)Sigma(g) ground electronic state. Our method is based on repeated optical pumping by laser light with a spectrum broad enough to excite all populated vibrational levels but limited in its frequency bandwidth with a spatial light modulator. In such a way we are able to eliminate transitions from the selected level, in which molecules accumulate. In this paper we briefly report the main experimental results and then address, in a detailed way by computer simulations, the perspectives for a \"complete\" cooling of the molecules, including also the rotational degree of freedom. Since the pumping process strongly depends on the relative shape of the ground and excited potential curves, ro-vibrational cooling through different excited states is theoretically compared.

Rivista/Giornale:  CHINESE JOURNAL OF CHEMICAL PHYSICS
Volume n.:  22 (2)      Pagine da: 149  a: 156
DOI: 10.1088/1674-0068/22/02/149-156

*Impact Factor della Rivista: (2009) 0.489   *Citazioni: 4
data tratti da "WEB OF SCIENCE" (marchio registrato di Thomson Reuters) ed aggiornati a:  19/05/2019

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